Irradiated Nuclear Fuel

Spent Fuel - Fuel Assembly
Typical fuel assembly

Irradiated nuclear fuel, also called the used nuclear fuel, is a nuclear fuel that has been irradiated in a nuclear reactor (usually at a nuclear power plant or an experimental reactor). Irradiated fuel, that can be considerred as spent fuel must be replaced by a fresh fuel due to its insufficient reactivity. Irradiated nuclear fuel is characterized by fuel burnup which is a measure of how much energy is extracted from a nuclear fuel and a measure of fuel depletion. Due to fuel depletion and fission fragments buildup, spent nuclear fuel is no longer useful in sustaining a nuclear reaction in an ordinary thermal reactor and it must be replaced by fresh fuel. Depending on its point along the nuclear fuel cycle, it may have considerably different isotopic constituents.

It must be noted, irradiated fuel is due to presence of high amount of radioactive fission fragments and transuranic elements very hot and very radioactive. Reactor operators have to manage the heat and radioactivity that remains in the “spent fuel” after it’s taken out of the reactor.  In nuclear power plants, spent nuclear fuel is usually stored underwater in the spent fuel pool on the plant.  Plant personnel move the spent fuel underwater from the reactor to the pool. Over time, as the spent fuel is stored in the pool, it becomes cooler as the radioactivity decays away. After several years (> 5 years), decay heat decreases under specified limits so that spent fuel may be reprocessed or interim storaged.

At first glance, it is difficult to recognize a fresh fuel from an used fuel. From mechanical point of view, the used fuel (irradiated) is identical as the fresh fuel. In most PWRs, used fuel assemblies stand between four and five metres high, are about 20 cm across and weighs about half a tonne. A PWR fuel assembly comprises a bottom nozzle into which rods are fixed through the lattice and to finish the whole assembly it is ended by a top nozzle. There are spacing grids between these nozzles. These grids ensure an exact guiding of the fuel rods. The bottom and top nozzles are heavily constructed as they provide much of the mechanical support for the fuel assembly structure. Western PWRs use a square lattice arrangement and assemblies are characterized by the number of rods they contain, typically, 17×17 in current designs. In contrast to the fresh fuel, which are simply shiny, the oxide layer forming on the surface of used fuel assemblies during the four-year fuel cycle makes them dark. Moreover,  Cherenkov radiation is typical only for spent nuclear fuel. The glow is visible also after the chain reaction stops (in the reactor). The cherenkov radiation can characterize the remaining radioactivity of spent nuclear fuel, therefore it can be used for measuring of fuel burnup.

Irradiated Nuclear Fuel – Burnup

As was written, spent nuclear fuel is characterized by fuel burnup, which defines energy release as well as it defines isotopic composition of irradiated fuel. Reactor engineers distinguish between:

  • Core Burnup. Averaged burnup over entire core (i.e. over all fuel assemblies). For example – BUcore = 25 000 MWd/tHM. This value do not characterizes spent fuel.
  • Fuel Assembly Burnup.  Averaged burnup over single assembly  (i.e. over all fuel pins of a single fuel assembly). For example – BUFA = 50 000 MWd/tHM. This value is typical for spent fuel.
  • Pin Burnup. Averaged burnup over single fuel pin or fuel rod (over all fuel pellets of a single fuel pin). For example – BUpin = 55 000 MWd/tHM. Fuel rods never have identical burnup. They slightly differ and limitations are set usually for fuel rod burnup due to fuel rod design considerations (e.g. internal pressure).
  • Local or Fine Mesh Burnup. Burnup significantly varies also within single fuel pellet. For example, the local burnup at the rim of the UO2 pellet can be 2–3 times higher than the average pellet burnup. This local anomaly causes formation of a structure known as High Burnup Structure.
References:
Nuclear and Reactor Physics:
  1. J. R. Lamarsh, Introduction to Nuclear Reactor Theory, 2nd ed., Addison-Wesley, Reading, MA (1983).
  2. J. R. Lamarsh, A. J. Baratta, Introduction to Nuclear Engineering, 3d ed., Prentice-Hall, 2001, ISBN: 0-201-82498-1.
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  5. W.S.C. Williams. Nuclear and Particle Physics. Clarendon Press; 1 edition, 1991, ISBN: 978-0198520467
  6. G.R.Keepin. Physics of Nuclear Kinetics. Addison-Wesley Pub. Co; 1st edition, 1965
  7. Robert Reed Burn, Introduction to Nuclear Reactor Operation, 1988.
  8. U.S. Department of Energy, Nuclear Physics and Reactor Theory. DOE Fundamentals Handbook, Volume 1 and 2. January 1993.

Advanced Reactor Physics:

  1. K. O. Ott, W. A. Bezella, Introductory Nuclear Reactor Statics, American Nuclear Society, Revised edition (1989), 1989, ISBN: 0-894-48033-2.
  2. K. O. Ott, R. J. Neuhold, Introductory Nuclear Reactor Dynamics, American Nuclear Society, 1985, ISBN: 0-894-48029-4.
  3. D. L. Hetrick, Dynamics of Nuclear Reactors, American Nuclear Society, 1993, ISBN: 0-894-48453-2. 
  4. E. E. Lewis, W. F. Miller, Computational Methods of Neutron Transport, American Nuclear Society, 1993, ISBN: 0-894-48452-4.

See above:

Spent Nuclear Fuel